I did read the Mars series as it came out.
Of course there were problems with creating a planitary enviornment on Mars where humans could live in the open atmosphere. Compared to attempting to remove the heavy metals and radioactive materials from Grayson, what they did in the Mars trilogy was childs play.
Heck, build up an human breathable atmosphere on Mars- which is more likely to take a millennia or so with technology we don't have yet and getting things to grow there (primarily things that photosynthesyse which is going to require a lot of water Mars donsn't have) plus creating that vast amount of carbon in gaseous form so the "plants" can create build celuar material will be interesting...not to mention where/how you are going to build up the free oxygen. There is the combined need to get enough atmosphear not only to provide air pressure as well as breathability but things like CO2 as a greenhouse effect -in this case to moderate the temperature swings. And that little problem of apparently not having a magnetic field similar to Earth'ss to help deflect solar particles etc. It goes on and on. There is also the small matter of producing food humans can eat prior to being able to plant out in that open atmosphere. The solution (quite interesting and actualy probable) in the film "The Martian" would be an initial approach but it will take a lot of shit and space (and sealable with heating and watered facilities) to do that.
Filter the natuarly accumulated heavy metals out of entire oceans, particularly when you are getting more diluted matrials draining into them from the rainfall on the land masses- ALL of the land masses and existing in ALL of the ocean and riverine sediment?
That is a fine engineering problem. At least Grayson seems to have a natual source of Oxygen in the atmosphere (which is also sort of balanced to an extent to which humans can breath it once you filter out all the things that will kill you with the dust and radiation.
But it is fiction. Barrayar seems to have found a possible solution for getting rid of radioactive problems from land from nuclear bombs (it's early days yet) but you would have to take that up with Louis McMaster Bujold